Thursday, 20 July 2017

Corrosive behaviour of Nickel based super alloys in Phosphoric Acid


For offering outstanding corrosion resistance and good mechanical characteristics, nickel based alloys are used in diverse applications in broad range of industries such as chemical, petrochemical processing, pollution control, oil and gas extraction, marine engineering, power production and pulp and paper manufacture. The versatility and reliability of these alloys make them special materials for construction of process vessels, pipes, pumps, valves and various other applications.

Pure phosphoric acid doesn’t possess any oxidizing power and is categorized as a non-oxidizing acid similar to dilute sulfuric. Commercial phosphoric acid although often consists of impurities of fluorides and chlorides that significantly make it corrosive. Oxidizing materials like ferric salts, may also be available to influence corrosion. Feasibly due to changes impurity concentrations of acids evaluated, studied corrosion rates are not always authenticated. Commonly used nickel alloys in processes of pure phosphoric acid are Incoloy 825 and Hastelloy G3.  In extreme hot phosphoric acid conditions, particularly those contaminated with halides, Inconel 625 is chosen.

Nickel 200 has limited significance in phosphoric acid. In pure, unaerated acid, corrosion rates are nominal for all acid concentrations at atmospheric temperatures. In hot or concentrated acid, corrosion rates are normally very high for using pure nickel.

Monel 400 offers significant resistance to pure phosphoric acid. Corrosion rates are below 10 mpy for all concentrations at temperatures up to 176oF or 80oC. Higher temperatures and aeration can considerably increase corrosion rates. Corrosion rates in crude phosphoric acid are very high due to presence of oxidizing salts. Even a nominal 0.4% ferric ion may accelerate the corrosion of an alloy.

Incoloy 825 offers great resistance to pure phosphoric acid at all concentrations and temperatures up to boiling 85% acid. Lab and plant corrosion test results are evaluated. In commercial grade phosphoric acid conditions, considerable pitting or crevice corrosion would limit the use of Incoloy alloy 825.

Inconel alloy 600 is resistant to phosphoric acid concentrations at room temperature. Although corrosion rates increase steeply with temperature therefore it is not recommended for use in warm acid.

Due to presence of high chromium and molybdenum concentrations and nominal magnitudes of niobium or tungsten, Alloy Inconel 625 wire and Hastelloy C276 offer outstanding resistance to phosphoric acid. In pure, concentrated, boiling acid, these alloys do not serve better than Incoloy 825. Although they show excellent resistance in the presence of significantly magnitudes of chlorides and fluorides that may cause pitting of Incoloy 825. Wet process acid evaporators are examples of these environments. In a solution of 25% phosphoric and 2% hydrofluoric acid at boiling point, Inconel 625 corroded at 2mpy in 48 hour test. Longer tests in practical operation have shown nominal corrosion rates and no localized corrosion in evaporating wet process phosphoric acid. The comparison of nickel based super alloys for corrosion resistance in commercially pure phosphoric acid in decreasing order is:

Hastelloy C276
Inconel 625
Incoloy 825

Monel 400

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