Sunday, 14 August 2016

Effect of heat processing on the welded Inconel 625’s corrosion resistance


Inconel 625 is an outstanding heat resistant alloy with good mechanical characteristics at the high temperatures and supreme corrosion resistance. These characteristics make it significant for use as a structural material in steam engines, nuclear plants and aircraft engines. It offers supreme welding properties and as a result it is used for weld overlay in the carbon steel pipes. Therefore it can be used instead high corrosion resistant steels for example duplex stainless steel. It also develops synergistic effect by weld overlay with carbon steel materials to supplement the yield strength of Inconel alloy and small corrosion resistance of carbon steel so it can be utilized as structural materials in the severe media like for example in crude oil. Moreover the heat expansion coefficients of the to metals are identical that decreases the chances of cracks due to thermal stress under the high temperature media. Although the Inconel alloy comprises of nickel and chromium, that may develop carbides and secondary phases, on the base of specific temperature and exposure time. Such carbides and secondary phases have a significant role in affecting the corrosion resistance and physical characteristics of alloy and causing the crack development. 

With the passage of time different carbides and secondary phases are developed that precipitate in the temperature limits from 600oC to 950oC. The development of these carbides can be a contributing aspect to the reduction of corrosion resistance. Intergranular regions of carbides are thermodynamically more inconsistent and highly active than other types of intergranulars. Intergranular regions increase owing to development of carbides. Additionally the carbides have higher chromium content than that present in the base metal. So when carbides are developed in the intergranular regions, the chromium content reduces around them resulting in to areas with low chromium content along the intergranualr regions. In this mechanism, chromium lacking areas are more prone to intergranular attack than other regions, so causing corrosion, is named as sensitization.
Electroslag welding method is implemented with alloy EQNiCrMo-3 utilized as a filler metal.

Aging
Aging heat processing was performed to find the intergranular resistance at 500A to 620A samples. Chromium carbides were developed through age heat processing at constant temperature for 100 hours in a vertical furnace at 850oC.

Corrosion tests
A single and double loop electrochemical reactivation test was performed as an electrochemical method to estimate the corrosion resistance. This test shows more significant results than with other chemicals. The sensitivity of intergranular attack on Inconel meals is assessed. The outcomes are assessed from non-uniform attack in the intergranular region and the outcomes should be evaluated by the current ratio. On the other hand, mistakes due to surface conditions are nominal and the test values can be easily received and compared with the single loop analysis. In high concentration of sulphuric acid, intergranular and other types of corrosion increases whilst in the low content, the corrosion is not noticed. So depending on the test condition factors, the tests are performed on nickel based alloy.

In the chemical analysis to evaluate the intergranular attack on stainless steel or  super alloy Inconel 625 plate, the tests included sulphate- sulphuric acid and nitric acid were performed. The ferric sulphate sulphuric acid test in the ASTM G28 method was conducted to assess the corrosion sensitivity of super alloys.
In the test of ferric sulphate sulphuric acid, H2SO4 acid solution comprising of 400 ml water and 236ml sulphuric acid where 25g dissolved Fe2(SO4)3 was utilized. It is warmed on a hot plate, the alloy sample was plunged for around 120 hours and the material loss was evaluated. To avoid evaporation of the solution beyond 120 hours, the boiling stone was kept in the solution and the vapour was condensed through flowing water condenser. The test results were received by substituting the noticed material loss of the samples.

In the another chemical test, the nitric acid test was performed that was aimed on evaluating the austenitic stainless steel and therefore was organized to fit the nickel based alloys in this analysis. Nickel super alloys have higher PREN than austenitic steel grades; the plunging period was increased up to 120 hours. In this test nitric acid is taken in 65% content.

No corrosion sign was found by intergranular attack on Inconel 625 due to its small carbon concentration and sufficiently high niobium magnitude. With small carbon concentration, chromium carbides, the main reason of chromium lacking regions, were not precipitated during aging heat processing, and with niobium effect, the niobium carbides were accumulated, hence preventing the development of chromium carbide. So the alloy was stabilized by precipitation along the grain. It is found that increased weight loss occurs with high heat supply to the sample. The weight loss in material is a crucial factor that shows the speed of corrosion as it results into the material degradation in the component.

Various corrosion rates are based on the type of attack. To determine this, microstructures of the corrosive surfaces were noticed after these chemical tests. The samples initially experienced corrosion at their intergranular regions. Initially thin and lengthy corrosion shape was seen however later the corrosion area increased and then at the maximum value of current the corrosion area becomes round. Alike outcomes were observed in the both tests.

Generally, the bigger weld heat supply, high dilution occurs in the weld metal and the base metal. With increase in weld heat supply, it results into melting a part of the main metal sample, therefore the metal’s atoms are diluted in the weld metal. It causes to increased diluted iron content in the weld metal hence decreasing the breaking potential. This iron dilution mechanism is noticed in the melted part and can also be seen in the fusion line zones by energy dispersive X ray spectroscopy. Increased niobium and molybdenum contents resulted into cracking. Therefore with increase in heat supply, the dilution effect is enhanced hence increasing iron concentration in the fusion line. As a result, large magnitude of iron was coagulated, initially in the dendritic regions, through weld solidification, niobium and molybdenum were emitted into the interdendritic regions. This method created microcrakcing in the dendritic and interdendritic regions, hence showing a variation in the corrosion resistance offered in these areas, and an unlike corrosion shape.

Outline
The samples were not found to be sensitive towards intergranular attack. Irrespective of nitrogen aging heat processing, precipitation of chromium carbide didn’t occur and niobium carbide stabilized the sample.


In the ferric sulfate sulphuric and nitric acid tests, heat supply improved with increase in material loss, hence corrosion rate is accelerated. 

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